N-(Diphenyl-carbamothio-yl)-3-methyl-benzamide

Document Type

Article

Publication Date

2-23-2009

Abstract

The synthesis of the title compound, C21H18N2OS, involves the reaction of 3-methyl-benzoyl chloride with potassium thio-cyanate in dry acetone followed by condensation of the 3-methyl-benzoyl isothio-cyanate with diphenyl-amine. The carbonyl [C - O = 1.215 (2) Å] and thio-carbonyl [C - S = 1.6721 (17) Å] distances indicate that these correspond to double bonds. The short C - N bonds at the center of the mol-ecule reveal the effects of resonance in this part of the mol-ecule. The conformation of the mol-ecule with respect to the thio-carbonyl and carbonyl groups is twisted. The 3-methyl-phenyl and two phenyl rings are also twisted, with dihedral angles of 75.67 (9) and 14.91 (9)°. The phenyl rings are rotated out of the mean plane of the N - C - S - N atoms by 66.87 (8) and 78.40 (9)°. Pairs of mol-ecules are linked into centrosymmetric dimers via inter-molecular N - H?S inter-actions and a C - H?O link also occurs. The dimers are stacked along the a axis.

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