Flame-retardant polypropylene/multiwall carbon nanotube nanocomposites: Effects of surface functionalization and surfactant molecular weight

Document Type

Article

Publication Date

1-1-2014

Abstract

Flame-retardant polypropylene (PP)/carbon nanotubes (CNTs) nanocomposites influenced by surface functionalization and surfactant molecular weights are studied. 3-Aminopropyl-triethoxysilane (APTES) is utilized to modify the CNTs (f-CNTs), and maleic-anhydride-grafted PP (MAPP) with two molecular weights (M?n of 800 and 8000 g mol-1) is used to further improve the dispersion of f-CNTs in the PP matrix. Thermal gravimetric analysis (TGA) and microscale combustion calorimetry (MCC) reveal that the molecular weight of MAPP directly affects the thermal stability and flammability of PP/f-CNTs PNCs: both MAPP polymers (M?n of 800 and 8000 g mol-1) increase the thermal stability of PP; however, the heat release rate of PP/f-CNTs is reduced in the presence of MAPP (M?n of 800 g mol-1) and increased in the presence of MAPP (M?n of 8000 g mol-1). MAPP (M?n of 800 g mol-1) also results in a lower viscosity of the PP/f-CNTs PNCs compared with pure PP. © 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

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